34 research outputs found
A new Raman technique of superior spectral resolution
Raman-active vibrational modes are coherently excited by the transient stimulated Raman process. A subsequent delayed probe of relatively long duration interacts with the freely relaxing vibrations. Raman spectra are generated with higher resolution and more accurate peak positions than in conventional Raman spectroscopy. In liquid cyclohexane four new Raman lines were readily detected in the frequency range 2870–2920 cm−1
Narrowing of spectral lines beyond the natural or dephasing line width
Transient excitation and gated or delayed observation provides a narrowing of the inherent line width of the transition. Possible experimental one- and two-photon systems are discussed and the loss of signal with line narrowing is calculated. The general case of lines broadened by dephasing processes is treated. Contact is made with the line narrowing in recent Raman type experiments
Quasi-particle Lifetimes in a d_{x^2-y^2} Superconductor
We consider the lifetime of quasi-particles in a d-wave superconductor due to
scattering from antiferromagnetic spin-fluctuations, and explicitly separate
the contribution from Umklapp processes which determines the electrical
conductivity. Results for the temperature dependence of the total scattering
rate and the Umklapp scattering rate are compared with relaxation rates
obtained from thermal and microwave conductivity measurements, respectively.Comment: 14 pages, 4 figure
The influence of phase-modulation on femtosecond time-resolved coherent Raman spectroscopy
The influence of phase-modulation on femtosecond time-resolved coherent Raman scattering is investigated theoretically and experimentally. The coherent Raman signal taken as a function of the spectral position shows unexpected temporal oscillations close to time zero. A theoretical analysis of the coherent Raman scattering process indicates that the femtosecond light pulses are amplitude and phase modulated. The pulses are asymmetric in time with more slowly decaying trailing wings. The phase of the pulse amplitude contains quadratic and higher-order contributions
Microwave conductivity of YBaCuO including inelastic scattering
The fluctuation spectrum responsible for the inelastic scattering in
YBaCuO which was recently determined from consideration of the
in-plane optical conductivity in the infrared, is used to calculate the
temperature dependence of the microwave conductivity at several measured
frequencies. Reasonable overall agreement can only be achieved if, in addition,
some impurity scattering is included within a model potential intermediate
between weak (Born) and strong (unitary) limit.Comment: 15 pages, 5 figures accepted for publication in Phys. Rev.
Dynamic structure selection and instabilities of driven Josephson lattice in high-temperature superconductors
We investigate the dynamics of the Josephson vortex lattice in layered
high-T superconductors at high magnetic fields. Starting from coupled
equations for superconducting phases and magnetic field we derive equations for
the relative displacements [phase shifts] between the planar Josephson arrays
in the layers. These equations reveal two families of steady-state solutions:
lattices with constant phase shifts between neighboring layers, starting from
zero for a rectangular configuration to for a triangular configuration,
and double-periodic lattices. We find that the excess Josephson current is
resonantly enhanced when the Josephson frequency matches the frequency of the
plasma mode at the wave vector selected by the lattice structure. The regular
lattices exhibit several kinds of instabilities. We find stability regions of
the moving lattice in the plane lattice structure - Josephson frequency. A
specific lattice structure at given velocity is selected uniquely by boundary
conditions, which are determined by the reflection properties of
electromagnetic waves generated by the moving lattice. With increase of
velocity the moving configuration experiences several qualitative
transformations. At small velocities the regular lattice is stable and the
phase shift between neighboring layers smoothly decreases with increase of
velocity, starting from for a static lattice. At the critical velocity
the lattice becomes unstable. At even higher velocity a regular lattice is
restored again with the phase shift smaller than . With increase of
velocity, the structure evolves towards a rectangular configuration.Comment: 28 pages, 12 figures, submitted to Phys. Rev.
Optical properties of the pseudogap state in underdoped cuprates
Recent optical measurements of deeply underdoped cuprates have revealed that
a coherent Drude response persists well below the end of the superconducting
dome. In addition, no large increase in optical effective mass has been
observed, even at dopings as low as 1%. We show that this behavior is
consistent with the resonating valence bond spin-liquid model proposed by Yang,
Rice, and Zhang. In this model, the overall reduction in optical conductivity
in the approach to the Mott insulating state is caused not by an increase in
effective mass, but by a Gutzwiller factor, which describes decreased coherence
due to correlations, and by a shrinking of the Fermi surface, which decreases
the number of available charge carriers. We also show that in this model, the
pseudogap does not modify the low-temperature, low-frequency behavior, though
the magnitude of the conductivity is greatly reduced by the Gutzwiller factor.
Similarly, the profile of the temperature dependence of the microwave
conductivity is largely unchanged in shape, but the Gutzwiller factor is
essential in understanding the observed difference in magnitude between ortho-I
and -II YBaCuO.Comment: 9 pages, 6 figures, submitted to Eur. Phys. J.
Optical Sum Rule anomalies in the High-Tc Cuprates
We provide a brief summary of the observed sum rule anomalies in the
high-T cuprate materials. A recent issue has been the impact of a
non-infinite frequency cutoff in the experiment. In the normal state, the
observed anomalously high temperature dependence can be explained as a `cutoff
effect'. The anomalous rise in the optical spectral weight below the
superconducting transition, however, remains as a solid experimental
observation, even with the use of a cutoff frequency.Comment: 4 pages, 2 figures, very brief review of optical sum rule anomal
Optical Sum Rule in Finite Bands
In a single finite electronic band the total optical spectral weight or
optical sum carries information on the interactions involved between the charge
carriers as well as on their band structure. It varies with temperature as well
as with impurity scattering. The single band optical sum also bears some
relationship to the charge carrier kinetic energy and, thus, can potentially
provide useful information, particularly on its change as the charge carriers
go from normal to superconducting state. Here we review the considerable
advances that have recently been made in the context of high oxides, both
theoretical and experimental.Comment: Review article accepted for publication in J. Low Temp. Phys. 29
pages, 33 figure